This study proposed a new curing agent consisting of slag and desulfurization gypsum industrial waste to solidify Cr(VI)-contaminated soils and prevent its migration and bioaccumulation in the ecosphere. The curing agent dosage of 10–30% resulted in a Cr(VI) toxic leaching concentration, compressive strength, and hydraulic conductivity range of 0.118–5.824 mg/L, 2.70–10.22 MPa, and 1.70 × 10−9–1.37 × 10−6 cm/s, respectively. Following four dry and wet cycles, the dosage of the curing agent was found to be 20–30% to achieve minimum envi...