Sorption-enhanced chemical looping steam reforming coupled with water splitting for syngas and H2 coproduction using waste plastic as fuel

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成果类型：

期刊论文

作者：

Zhong, Mingxuan;Cai, Yongcheng;Wang, Chenxuanzi;Li, Jianfen;Xiao, Bo;...

通讯作者：

Xu, TT;Wang, X

作者机构：

[Li, Jianfen; Cai, Yongcheng; Zhong, Mingxuan; Wang, Chenxuanzi; Wang, Xun; Xiao, Bo] Huazhong Univ Sci & Technol, Sch Environm Sci & Engn, Hubei Key Lab Multimedia Pollut Cooperat Control Y, 1037 Luoyu Rd, Wuhan 430074, Hubei, Peoples R China.

[Li, Jianfen; Cai, Yongcheng; Zhong, Mingxuan; Wang, Chenxuanzi; Wang, Xun; Xiao, Bo] Huazhong Univ Sci & Technol, Green Energy Ind Res Ctr GEIRC, 1037 Luoyu Rd, Wuhan 430074, Hubei, Peoples R China.

[Li, Jianfen] Wuhan Polytech Univ, Sch Chem & Environm Engn, Wuhan 430023, Peoples R China.

[Xu, Tingting] Nanjing Univ Sci & Technol, Sch Energy & Power Engn, MIIT Key Lab Thermal Control Elect Equipment, Nanjing 210094, Peoples R China.

[Xu, TT] Nanjing Univ Sci & Technol, Sch Energy & Power Engn, Nanjing 210094, Peoples R China.

通讯机构：

[Xu, TT ] N

[Wang, X ] H

Nanjing Univ Sci & Technol, Sch Energy & Power Engn, Nanjing 210094, Peoples R China.

Huazhong Univ Sci & Technol, Sch Environm Sci & Engn, Wuhan 430074, Peoples R China.

语种：

英文

关键词：

Sorption-enhanced technology;Chemical looping steam reforming;Hydrogen production;Waste plastic;Brownmillerite

期刊：

Chemical Engineering Journal

ISSN：

1385-8947

年：

2024

卷：

494

页码：

152927

DOI：

10.1016/j.cej.2024.152927

基金类别：

CRediT authorship contribution statement Mingxuan Zhong: Writing – review & editing, Writing – original draft, Visualization, Software, Investigation, Conceptualization. Yongcheng Cai: Software, Methodology, Conceptualization, Writing – original draft. Chenxuanzi Wang: Visualization, Methodology, Formal analysis. Jianfen Li: Writing – review & editing. Bo Xiao: Conceptualization. Tingting Xu: Investigation, acquisition. Xun Wang: Writing – review & editing, Supervision, acquisition, Conceptualization.

机构署名：

本校为其他机构

院系归属：

化学与环境工程学院

摘要：

Chemical looping is a promising technology for hydrogen production. Achieving both high purity and yield is an ongoing challenge, due to low fuel conversion and carbon deposition. In this study, a sorption-enhanced chemical looping reforming coupled with water splitting (SE-CLSR-WS) process was proposed to co-produce syngas and H 2 by using waste plastic as the fuel. The Ni-doped Ca 2 Fe 2 O 5 brownmillerites were designed and employed as oxygen carriers (OCs) and CO 2 sorbent. The introduction of Ni leaded to lattice distortion of brownmillerite, thereby enhancing the redox activity of lattic...

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Sorption-enhanced chemical looping steam reforming coupled with water splitting for syngas and H2 coproduction using waste plastic as fuel

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