Defect engineering on metal-organic frameworks for enhanced photocatalytic reduction of Cr(VI)

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成果类型：

期刊论文

作者：

Ma, Jiaqi;Fan, Linkun;Wang, Xusheng*;Li, Lan;Zhang, Yiming;...

通讯作者：

Wang, Xusheng;Gao, JK

作者机构：

[Fan, Linkun; Gao, JK; Wang, Xusheng; Wang, XS; Gao, Junkuo; Ma, Jiaqi] Zhejiang Sci Tech Univ, Sch Mat Sci & Engn, Hangzhou 310018, Peoples R China.

[Wang, Xusheng] Zhejiang Sci Tech Univ, Shengzhou Innovat Res Inst, Shengzhou 312400, Zhejiang, Peoples R China.

[Wang, Xusheng] Jinan Univ, Guangdong Prov Key Lab Funct Supramol Coordinat Ma, Guangzhou 510632, Peoples R China.

[Li, Lan] China Jiliang Univ, Coll Mat & Chem, Hangzhou 310018, Peoples R China.

[Zhang, Yiming] Lanzhou Univ Technol, Sch Mat Sci & Engn, Lanzhou 730050, Peoples R China.

通讯机构：

[Gao, JK ; Wang, XS] Z

Zhejiang Sci Tech Univ, Sch Mat Sci & Engn, Hangzhou 310018, Peoples R China.

语种：

英文

关键词：

Metal-organic frameworks;Oxygen vacancy;Mesoporous structure;Heat treatment;Defect

期刊：

Surfaces and Interfaces

ISSN：

2468-0230

年：

2024

卷：

页码：

105174

DOI：

10.1016/j.surfin.2024.105174

基金类别：

CRediT authorship contribution statement Jiaqi Ma: Writing – review & editing, Writing – original draft, Visualization, Investigation. Linkun Fan: Writing – original draft, Visualization, Investigation. Xusheng Wang: Writing – review & editing, Supervision, Project administration, acquisition, Conceptualization. Lan Li: Investigation. Yiming Zhang: Investigation. Guixia Zhao: Investigation. Bo Chai: Investigation. Junkuo Gao: Writing – review & editing, Resources, acquisition.

机构署名：

本校为其他机构

院系归属：

化学与环境工程学院

摘要：

Cr(VI) stands as a profoundly toxic chemical and photocatalysis technology has shown promising potential in photocatalytic reduction of Cr(VI) to Cr(III), where the reduced Cr(III) is less toxic and can be further precipitated in a wide pH range. Metal-organic frameworks (MOFs), as emerging class of porous coordination polymers, is expected to be ideal platform for photocatalysis. In this study, defect engineering on MOFs was applied to promote photoreduction of Cr(VI). The obtained oxygen vacancy-containing MIL-125-NH2 samples showed modified ...

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Defect engineering on metal-organic frameworks for enhanced photocatalytic reduction of Cr(VI)

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