Atomically dispersed cobalt activator with nitrogen and sulfur co-coordination for high-efficiency Fenton-like catalysis: Insights into density-dependent activity and mechanisms

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作者信息关键词期刊信息基础信息归属信息摘要

成果类型：

期刊论文

作者：

Long, Yangke*;Zhao, Jiakun;Dai, Jian;Lu, Guangzhao;Lin, Manling;...

通讯作者：

Long, Yangke;Li, Sheng

作者机构：

[Long, Yangke] Department of Transportation and Environment, Shenzhen Institute of Information Technology, Shenzhen 518172, China. Electronic address: longyk@sziit.edu.cn

[Zhao, Jiakun] School of Chemical and Environmental Engineering, Wuhan Polytechnic University, Wuhan 430023, China

[Dai, Jian] School of Instrumentation Science and Engineering, Harbin Institute of Technology, Harbin 150080, China

[Lin, Manling; Lu, Guangzhao] Department of Transportation and Environment, Shenzhen Institute of Information Technology, Shenzhen 518172, China

[Li, Sheng] School of Chemical and Environmental Engineering, Wuhan Polytechnic University, Wuhan 430023, China. Electronic address: lfrcs@163.com

通讯机构：

[Li, Sheng] S

[Long, Yangke] D

Department of Transportation and Environment, Shenzhen Institute of Information Technology, Shenzhen 518172, China. Electronic address:

School of Chemical and Environmental Engineering, Wuhan Polytechnic University, Wuhan 430023, China. Electronic address:

语种：

英文

关键词：

Activation mechanisms;Emerging organic contaminants;Metal leaching;Oxidative degradation;Sub-nanometric catalysts

期刊：

Journal of Hazardous Materials

ISSN：

0304-3894

年：

2024

卷：

469

页码：

133996

DOI：

10.1016/j.jhazmat.2024.133996

机构署名：

本校为通讯机构

院系归属：

化学与环境工程学院

摘要：

Atomically dispersed metal activators (ADMAs) have demonstrated unique advantages in environmental remediation, but how to controllably regulate the active site density and electronic structure of ADMAs to further enhance activation efficiency remains challenging. Here, we introduce a sulfur-atom-doping approach that allows the fine-tuning of atomic Co site content and electronic structure, enabling exploration of density-dependent activation performance of ADMAs for peroxymonosulfate (PMS)-based Fenton-like catalysis. Our investigation reveals...

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Atomically dispersed cobalt activator with nitrogen and sulfur co-coordination for high-efficiency Fenton-like catalysis: Insights into density-dependent activity and mechanisms

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