Reconstruction of Bi2S3 in CO2 Electroreduction via Topotactic Transformation - 成果

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Reconstruction of Bi₂S₃ in CO₂ Electroreduction via Topotactic Transformation

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成果类型：

期刊论文

作者：

Ding, Yunxuan;Li, Yaqing;Wang, Linqin;Chai, Bo;Jia, Yufei;...

通讯作者：

Sun, LC;Sun, Licheng;Fan, K

作者机构：

[Sun, LC; Sun, Licheng; Ding, Yunxuan; Wang, Linqin] Westlake Univ, Ctr Artificial Photosynth Solar Fuels, Sch Sci & Res Ctr Ind Future, Hangzhou 310024, Peoples R China.

[Chai, Bo] Wuhan Polytech Univ, Sch Chem & Environm Engn, Wuhan 430023, Peoples R China.

[Sun, LC; Sun, Licheng; Ding, Yunxuan; Wang, Linqin] Westlake Univ, Res Ctr Ind Future, Sch Sci, Dept Chem, Hangzhou 310024, Peoples R China.

[Sun, LC; Sun, Licheng; Ding, Yunxuan; Wang, Linqin] Westlake Univ, Div Solar Energy Convers & Catalysis, Zhejiang Baima Lake Lab Co Ltd, Hangzhou 310000, Zhejiang, Peoples R China.

[Jia, Yufei; Fan, Ke; Sun, Licheng; Sun, LC; Li, Yaqing] Dalian Univ Technol, DUT KTH Joint Educ & Res Ctr Mol Devices, Inst Artificial Photosynth,Frontier Sci Ctr Smart, Inst Energy Sci & Technol,State Key Lab Fine Chem, Dalian 116024, Peoples R China.

通讯机构：

[Fan, K ; Sun, LC] D

[Sun, LC ] W

Westlake Univ, Ctr Artificial Photosynth Solar Fuels, Sch Sci & Res Ctr Ind Future, Hangzhou 310024, Peoples R China.

Westlake Univ, Res Ctr Ind Future, Sch Sci, Dept Chem, Hangzhou 310024, Peoples R China.

Westlake Univ, Div Solar Energy Convers & Catalysis, Zhejiang Baima Lake Lab Co Ltd, Hangzhou 310000, Zhejiang, Peoples R China.

语种：

英文

关键词：

topotactic transformation;CO2 reduction;Bi2S3;morphology;formate

期刊：

ACS Applied Energy Materials

ISSN：

2574-0962

年：

2024

卷：

期：

页码：

5418-5425

DOI：

10.1021/acsaem.4c00716

基金类别：

National Key Research and Development Program of China#&#&#2022YFA0911904 Fundamental Research Funds for the Central Universities#&#&#DUT23LAB611 National Natural Science Foundation of China#&#&#22088102 Fundamental Research Center of Artificial Photosynthesis

机构署名：

本校为其他机构

院系归属：

化学与环境工程学院

摘要：

Bismuth-based catalysts have demonstrated significant electrocatalytic activity in the electrochemical CO2 reduction reaction (CO2RR) to produce formate/formic acid, while the morphology of these catalysts is considered to be crucial for their electrocatalytic performance. However, the potential topological transformation of Bi-based catalysts during CO2RR catalysis has been largely overlooked, which could lead to an underlying lack of understanding of the structure-activity relationship. In this study, various morphologies of bismuth sulfide (Bi2S3), including nanowires, nanoribbons, nanosphe...

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Reconstruction of Bi₂S₃ in CO₂ Electroreduction via Topotactic Transformation

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