Highly-dispersed CdS nanoparticles coating hierarchical Ni@NC derived from ultrathin nanosheets NMOF-Ni: Photocatalytic hydrogen evolution coupled with alcohol oxidation

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成果类型：

期刊论文

作者：

Yang, Heng;Xia, Yang;Guo, Jie;Xue, Lu;Carabineiro, Sonia A. C.;...

通讯作者：

Wen, LL

作者机构：

[Wen, LL; Guo, Jie; Yang, Heng; Xue, Lu; Wen, Lili; Ouyang, Shuxin] Minist Educ, Engn Res Ctr Photoenergy Utilizat Pollut Control, Wuhan 430079, Peoples R China.

[Wen, LL; Guo, Jie; Yang, Heng; Xue, Lu; Wen, Lili; Ouyang, Shuxin] Cent China Normal Univ, Coll Chem, Wuhan 430079, Peoples R China.

[Yang, Heng] Wuhan Polytech Univ, Coll Chem & Environm Engn, Wuhan, Peoples R China.

[Xia, Yang] Wuhan Inst Technol, Sch Chem Engn & Pharm, Minist Educ, Key Lab Green Chem Engn Proc, Wuhan 430072, Peoples R China.

[Carabineiro, Sonia A. C.] Univ NOVA Lisboa, NOVA Sch Sci & Technol, Dept Chem, LAQV REQUIMTE, P-2829516 Caparica, Portugal.

通讯机构：

[Wen, LL ] M

Minist Educ, Engn Res Ctr Photoenergy Utilizat Pollut Control, Wuhan 430079, Peoples R China.

Cent China Normal Univ, Coll Chem, Wuhan 430079, Peoples R China.

语种：

英文

关键词：

Dual-functional photocatalyst;Photocatalytic H-2 evolution;Selective oxidation of alcohols;Ultrathin nanosheets-derived Ni@NC;Hierarchical structure

期刊：

Applied Catalysis B: Environment and Energy

ISSN：

0926-3373

年：

2025

卷：

362

页码：

124700

DOI：

10.1016/j.apcatb.2024.124700

基金类别：

National Nature Science Foundation of China [22171097, 21771072, 22402156, 22108211]; Fundamental Research Funds for the Central Universities [CCNU22QN008]; Research and Innovation Initiatives of WHPU [2024Y18]

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院系归属：

化学与环境工程学院

摘要：

Photocatalytic water-splitting into H 2 in conventional procedures often requires sacrificial agents to consume unutilized holes to boost the reaction. Herein, we cast off the dependence on the addition of sacrificial agents and develop a dual-functional photocatalyst CdS/Ni@NC for coupling H 2 evolution with value-added benzyl alcohol (BA) oxidation in anaerobic aqueous solution, wherein CdS/Ni@NC was synthesized by in-situ anchoring of CdS nanoparticles (NPs) onto NMOF-Ni ultrathin nanosheets-derived nitrogen-doped wrinkled graphitic carbon l...

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Highly-dispersed CdS nanoparticles coating hierarchical Ni@NC derived from ultrathin nanosheets NMOF-Ni: Photocatalytic hydrogen evolution coupled with alcohol oxidation

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