Precise Cation Recognition in Two-Dimensional Nanofluidic Channels of Clay Membranes Imparted from Intrinsic Selectivity of Clays

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成果类型：

期刊论文

作者：

Zhang, Tingting;Bai, Haoyu*;Zhao, Yunliang;Ren, Bo;Wen, Tong;...

通讯作者：

Bai, Haoyu;Zhao, YL;Bai, HY

作者机构：

[Zhang, Tingting] Wuhan Polytech Univ, Sch Chem & Environm Engn, Wuhan 430023, Hubei, Peoples R China.

[Bai, Haoyu; Chen, Licai; Zhao, YL; Ren, Bo; Zhao, Yunliang; Song, Shaoxian; Wen, Tong] Wuhan Univ Technol, Sch Resources & Environm Engn, Wuhan 430070, Hubei, Peoples R China.

[Bai, Haoyu; Chen, Licai; Zhao, YL; Ren, Bo; Zhao, Yunliang; Song, Shaoxian; Wen, Tong] Wuhan Univ Technol, Hubei Key Lab Mineral Resources Proc & Environm, Wuhan 430070, Hubei, Peoples R China.

[Bai, Haoyu] Imperial Coll London, Dept Mat, London SW7 2AZ, England.

[Komarneni, Sridhar] Penn State Univ, Dept Ecosyst Sci & Management, Energy & Environm Lab 204, University Pk, PA 16802 USA.

通讯机构：

[Bai, HY; Zhao, YL ] W

[Bai, HY ] I

Wuhan Univ Technol, Sch Resources & Environm Engn, Wuhan 430070, Hubei, Peoples R China.

Wuhan Univ Technol, Hubei Key Lab Mineral Resources Proc & Environm, Wuhan 430070, Hubei, Peoples R China.

Imperial Coll London, Dept Mat, London SW7 2AZ, England.

语种：

英文

关键词：

2D nanofluidic channels;clay nanosheets;structural modification;ionic selectivity;clay membranes;separation of lithium and magnesium

期刊：

ACS Nano

ISSN：

1936-0851

年：

2022

卷：

期：

页码：

4930-4939

DOI：

10.1021/acsnano.2c00866

基金类别：

The financial support for this work from the National Natural Science Foundation of China (Nos. 51904215 and 51874220), Natural Science Foundation of Hubei Province of China (2021CFB554), and the Fundamental Research Funds for the Central Universities (WUT: 2020IVB016, 2021-zy-028) is gratefully acknowledged. H.B. greatly acknowledges the financial support provided by China Scholarship Council (CSC)-Imperial Scholarship (CSC No. 202106950021).

机构署名：

本校为第一机构

院系归属：

化学与环境工程学院

摘要：

Various kinds of clays occur naturally and are accompanied by particular cations in their interlayer domains. Here we report the reassembled membranes with nanofluidic channel arrays by using the natural clays montmorillonite, mica, and vermiculite, which were imparted with the natural selectivity for realizing precise recognition and directional regulation of the naturally occurring interlayer cations. A typical surface-governed ionic transport behavior was observed in the clay nanofluidic channels. Through asymmetric structural modification, ...

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Precise Cation Recognition in Two-Dimensional Nanofluidic Channels of Clay Membranes Imparted from Intrinsic Selectivity of Clays

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