Efficient activation of peroxymonosulfate for catalytic degradation of organic pollutants by simultaneously using low-level cobalt ions and calcium carbonate micro-particles

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成果类型：

期刊论文

作者：

Zhou, Yu;Wang, Xiaobo;Wang, Nan;Huang, Shuangshuang;Zhu, Lihua

通讯作者：

Xiaobo Wang<&wdkj&>Lihua Zhu

作者机构：

[Zhou, Yu; Wang, Nan; Zhu, Lihua] College of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan, 430074, China

College of Chemistry and Chemical Engineering, Hubei Polytechnic University, Huangshi, 435003, China

College of Chemistry and Environmental Engineering, Wuhan Polytechnic University, Wuhan, 430023, China

[Huang, Shuangshuang] School of Physics and Technology, Center for Electron Microscopy, Wuhan University, Wuhan, China

[Wang, Xiaobo] College of Chemistry and Chemical Engineering, Hubei Polytechnic University, Huangshi, 435003, China<&wdkj&>College of Chemistry and Environmental Engineering, Wuhan Polytechnic University, Wuhan, 430023, China

通讯机构：

[Xiaobo Wang; Lihua Zhu] C

College of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan 430074, China<&wdkj&>College of Chemistry and Chemical Engineering, Hubei Polytechnic University, Huangshi 435003, China<&wdkj&>College of Chemistry and Environmental Engineering, Wuhan Polytechnic University, Wuhan 430023, China

语种：

英文

关键词：

Aromatic compounds;Benzoic acid;Calcite;Catalyst activity;Chemical activation;Chemicals removal (water treatment);Cobalt compounds;Heavy metals;Metal ions;Organic pollutants;Rate constants;Wastewater treatment;Catalytic degradation;Catalytic system;Cobalt ion;Low-level cobalt;Methylene Blue;Micro particles;Oxidative degradation;Peroxymonosulfate;Peroxymonosulfate activations;Synergistic effect;Calcium carbonate;calcium carbonate;catalyst;cobalt;ion exchange;organic pollutant;wastewater treatment

期刊：

环境科学学报(英文版)

ISSN：

1001-0742

年：

2025

卷：

151

页码：

113-124

DOI：

10.1016/j.jes.2024.04.004

基金类别：

The authors acknowledge the funding supports from thes National Natural Science Foundation of China (Nos. 22076052 and 21976063 ) and from China Postdoctoral Science Foundation (No. 2018M642850 ); Research Funding of Wuhan Polytechnic University (NO. 2023RZ017 ).

机构署名：

本校为通讯机构

院系归属：

化学与环境工程学院

摘要：

An efficient catalytic system was developed to remove various organic pollutants by simultaneously using low-level cobalt ions, calcium carbonate micro-particles and peroxymonosulfate (PMS). A simple base-induced precipitation was used to successfully loaded Co-centered reactive sites onto the surface of CaCO3 microparticles. Under optimal conditions at 25 °C, 10 mg/L methylene blue (MB) could be completely degraded within 10 min with 480 µg/L Co2+, 0.4 g/L CaCO3 microparticles (or 0.4 g/L Co@CaCO3) and 0.1 g/L PMS. The MB degradation followe...

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Efficient activation of peroxymonosulfate for catalytic degradation of organic pollutants by simultaneously using low-level cobalt ions and calcium carbonate micro-particles

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