The inherent properties of TiO(2), including a wide band gap and restricted spectral response range, hinder its commercial application and its ability to harness only 2-3% of solar energy. To address these challenges and unlock TiO(2)'s full potential in photocatalysis, C(60)- and CdS-co-modified nano-titanium dioxide has been adopted in this work to reduce the band gap, extend the absorption wavelength, and control photogenerated carrier recombination, thereby enhancing TiO(2)'s light-energy-harnessing capabilities and hydrogen evolution capac...